| Date | VT Rank | Opponent | Result | TV | Location |
|---|---|---|---|---|---|
| Sat., Sep 17, 1966 | at Tulane | L, 0-13 | New Orleans, La. | ||
| Sat., Sep 24, 1966 | George Washington | W, 49-0 | Blacksburg, Va. | ||
| Sat., Oct 1, 1966 | West Virginia | T, 13-13 | Blacksburg, Va. | ||
| Sat., Oct 8, 1966 | at Kentucky | W, 7-0 | Lexington, Ky. | ||
| Sat., Oct 15, 1966 | vs. Vanderbilt | W, 21-6 | Richmond, Va. | ||
| Sat., Oct 22, 1966 | at Virginia | W, 24-7 | Charlottesville, Va. | ||
| Homecoming | |||||
| Sat., Oct 29, 1966 | Florida State | W, 23-21 | ABC (regional) | Blacksburg, Va. | |
| Sat., Nov 5, 1966 | at Wake Forest | W, 11-0 | Winston-Salem, N.C. | ||
| Sat., Nov 12, 1966 | at William & Mary | W, 20-18 | Williamsburg, Va. | ||
| Thu., Nov 24, 1966 | vs. VMI | W, 70-12 | Roanoke, Va. | ||
| Liberty Bowl | |||||
| Sat., Dec 10, 1966 | vs. #9 Miami | L, 7-14 | ABC (national) | Memphis, Tenn. | |
| Overall: 8-2-1 Conference: 0-0 Home: 2-0-1 Away: 4-1 Neutral: 2-1 |
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